- A.B. Akard Collection, c.1916 and 1937
- Panoramic Photograph of Broad Street Methodist Church, undated
- .54 Caliber Bullet, c. 1864
- A Group of Citizens Interested in Just and Equal Law Enforcement (Political Broadside), c. 1958.
- Account Sheets from Eastman and Peerless Coal Companies, 1938-1947
- Aerial View of the Granby Road and Vulcan Materials Company Area, c. 1970s
- Alvin C. York Photograph, post World War I
- American Association of Retired Persons (AARP), Greater Kingsport Chapter 3109 Collection, 1977-1991
- American Association of University Women Collection (Kingsport, Tennessee Branch), 1947-1999
- American History Project Collection, c. 1943
- American Legion Hammond Post, No. 3 Decorating Committee Collection, 1969-1970
- American Red Cross of Northeast Tennessee Collection, 1946-ongoing
- Ann K. Morison Collection, 1847-2003
- Anna Doggett Cannon Collection, c.1886-1977
- Anna Lou Crumley Photograph, 1929
- Annie Mitchell Papers, 1902-1929
- Appalachian Fair Booklet, August 23-28, 1976
- Bachelder’s Studio and McLean Studio Photographs, c. January 1916 and 1925
- Bacon, Fulkerson, and Moore Families Papers, 1927-1945
- Baltimore & Ohio Railroad Company Ledger, July 1899-May 1900
- Bank of Kingsport Collection, 1910
- Barnes and Bridwell Families Photograph, c. 1920s
- Bays Mountain Park Records, 1926-ongoing
- Belt Chatter, May 1928
- Betsy Boyd Homecoming ’86 Materials, 1985-1988
- Bill Ford Collection, undated
- Blanche McMillan Collection, May 7, 1930
- Blue Ridge Garden Club Records, 1953-1978
- Boatyard Cemetery Maintenance Collection, October 1988
- Bob Lawrence Kingsport Postcard Collection, c. 1940s
- Bobby Dodd Coach of the Year Foundation Records, 2002-2004.
- Borden Mills and J.P. Stevens Companies Collection, 1948-1988
- Bratton & Co. Ledger, 1888-1891
- Business and Professional Women of Kingsport Records, 1940-2005
- C. James Frye Collection, c.1918-c.1942
- Calvin Fitzwater Collection, 1921-2003
- Carl Swann Collection, 1930-1974
- Carolina, Clinchfield and Ohio Railroad Photographs,1909-1922
- Charles Andrew and Ernestine E. Bernard Postcard Collection, 1934-1959
- Cherry Hill Disaster, Sheet Music, undated
- Church Circle on Christmas Eve Painting, undated
- Church Directories and Histories, 1961-1999
- Church Women United, Kingsport Branch Collection, 1933-2004
- Circle Churches Christmas Foundation By-Laws and Minutes, July-August 1966
- Civilian Conservation Corps Photographs, mid 1930s
- Claude S. Jones Collection, 1931-1987
- Clifford Family Scrapbooks, c. 1915-early 1920s
- Clinchfield Railroad Steam Freight Train Photograph (copy), April 16, 1954.
- Clyde Mitchell Collection, 1937-1999 and undated
- Collection of Glass Plate Negatives and Slides, 1920s and undated
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